Let us know when you're done.
Seriously, tho, I would imagine this would be as difficult as finding a precise ballistic coeficient. What with the various bullet lengths, densities, nose profiles, etc. to consider, determining an exact optimum spin would be damn-near impossible; it's kind of tough to measure the air pressures around a particular bullet as it cuts through the air, so we really don't have any idea of what's really going on. It's pretty tough to come up with an accurate mathematical model in the general absence of data.
Greenhill's formula was hatched at a point in time where all bullets left their respective barrels at pretty much the same velocity (owing to the pressure limitations of black powder), and all bullets looked pretty much the same (round nose, 1-3 calibers long). The formula was a general mathematical guide, and at the time, worked reasonably well. Things now are a bit more complicated , no?